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李喜林, 刘思初, 吴美林, 高梦晴, 谷 庆, 刘思源, 李嘉宁, 王 健.羟基磷灰石同步去除地下水中氟、铁和锰性能水资源与水工程学报[J].,2021,32(6):27-34
羟基磷灰石同步去除地下水中氟、铁和锰性能
Synchronous adsorption of fluorine, iron and manganese from groundwater by hydroxyapatite
  
DOI:10.11705/j.issn.1672-643X.2021.06.04
中文关键词:  羟基磷灰石        同步吸附  表面络合  离子交换
英文关键词:hydroxyapatite  fluorine  iron  manganese  synchronous adsorption  surface complexation  ion exchange
基金项目:国家重大研发计划重点专项(2017YFC1503100); 辽宁省教育厅科学研究面上项目(LJKZ0344); 辽宁省百千万人才工程项目(2018C01); 辽宁省大学生创新性实验计划项目(S202010147028)
作者单位
李喜林, 刘思初, 吴美林, 高梦晴, 谷 庆, 刘思源, 李嘉宁, 王 健 (辽宁工程技术大学 土木工程学院 辽宁 阜新 123000) 
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中文摘要:
      为解决含氟、铁和锰地下水对人类生活和身体健康带来的危害,采用溶胶凝胶法合成羟基磷灰石,运用单因素轮转法找到最佳吸附性能参数,建立等温吸附模型及吸附动力学方程,采用SEM、EDS、XRD和FTIR微观表征方法分析吸附机理,并对羟基磷灰石的再生循环性及实际应用性进行研究。结果表明:羟基磷灰石最佳吸附条件为投加量4 g/L、反应时间150 min、反应温度35 ℃,此时,对试验水样中F-、Fe2+、Mn2+的去除率分别为84.6%、99.9%和99.8%,达到《生活饮用水卫生标准》(GB 5749—2006)要求。羟基磷灰石对氟、铁和锰的吸附均符合Langmuir等温吸附,且吸附是自发的吸热熵增过程,吸附过程符合准二级动力学方程。羟基磷灰石通过物理吸附、表面络合反应和离子交换作用可以实现对地下水中F-、Fe2+以及Mn2+的同步吸附去除。
英文摘要:
      In order to reduce the harm of groundwater containing fluorine, iron and manganese to the livelihood of human lives, hydroxyapatite was synthesized by sol-gel method for the adsorption of these elements. The optimal adsorption performance parameters were selected by single factor rotation method to establish an isothermal adsorption model and adsorption kinetics equation. Then, the adsorption mechanism was analyzed by SEM, EDS, XRD and FTIR microscopic characterization methods, and the recycling property and practical application of hydroxyapatite were studied. The results show that the optimal adsorption conditions of hydroxyapatite are as follows: the dosage is 4 g/L, the reaction time is 150 min, and the reaction temperature is 35 ℃. Under these conditions, the removal rates of F-, Fe2+, and Mn2+ in the test water samples were 84.6%, 99.9%, and 99.8%, respectively, which met the requirements of standards for drinking water quality (GB 5749—2006).The adsorption of fluoride, iron and manganese by hydroxyapatite is in line with Langmuir isothermal adsorption, and the adsorption is a spontaneous endothermic entropy increase process, which conforms to the pseudo-second-order kinetic equation. The application of hydroxyapatite can achieve simultaneous adsorption and removal of F-, Fe2+, and Mn2+ in groundwater through physical adsorption, surface complexation reaction and ion exchange.
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