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李晓刚, 赵良菊, 刘 琼, 赵咏琪, 成 静, 卢久菊, 赵培琦.秦岭山区商洛市大气降水化学组成特征及来源分析水资源与水工程学报[J].,2020,31(4):24-30
秦岭山区商洛市大气降水化学组成特征及来源分析
Chemical composition of precipitation and its sources in Shangluo City of Qinling mountainous area
  
DOI:10.11705/j.issn.1672-643X.2020.04.04
中文关键词:  城市降水; 化学组成; 离子来源; 秦岭山区  商洛市
英文关键词:urban precipitation  chemical composition  ion sources  Qingling mountainous area  Shangluo City
基金项目:国家自然科学基金项目(41701090); 陕西省创新能力支撑计划项目(2019KJXX-026); 陕西省教育厅科学研究项目(18JK0245); 陕西省大学生创新创业训练项目(S201911396024);商洛学院科研项目(18SKY002)
作者单位
李晓刚1, 赵良菊2, 刘 琼1, 赵咏琪1, 成 静1, 卢久菊1, 赵培琦1 (1.商洛学院 城乡规划与建筑工程学院 陕西 商洛726000 2.西北大学 城市与环境学院 陕西 西安710127) 
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中文摘要:
      为了解秦岭山区城市大气降水化学组成与来源,2018年1-12月共收集商洛市有效降水样品40个,分析了pH、电导率(EC)和主要离子浓度(F- 、Cl-、NO-3、SO42-、NH4+、K+、Na+、Ca2+和Mg2+)。结果表明:商洛市降水pH和电导率的加权平均值分别为6.76和34.35 μS/cm,降水总离子浓度加权平均值为452.89 μeq/L;主要阴离子为SO42-和NO-3,分别占总阴离子浓度的59.20%和31.93%,主要阳离子为NH4+和Ca2+,分别占阳离子浓度的39.21%和33.87%,中和因子(NF)也表明二者中和能力最强;总离子浓度冬季高,夏秋季低,呈现明显的季节变化特征;相关分析表明NH4+、Ca2+与SO42-、NO-3之间相关系数均大于0.7,说明商洛大气中存在着NH4NO3、Ca(NO3)2、(NH4)2SO4、CaSO4和NH4HSO4等物质;富集因子计算表明,SO42-和NO-3主要来自人为活动,Ca2+、Mg2+和K+主要来自陆源的岩石土壤风化,Cl-主要来自于海洋源。
英文摘要:
      To better understand the characteristics and sources of chemical composition of urban precipitation in Qinling mountainous area, we collected 40 precipitation samples from January to December, 2018 to analyze the values of pH, electrical conductivity (EC) and the concentration of main ions (F- , Cl-, NO-3, SO42-, NH4+, K+, Na+, Ca2+ and Mg2+). The results showed that the weighted means of pH and EC in the precipitation samples were 6.76 and 34.35 μS/cm respectively. The weighted mean of total ion concentration in the precipitation samples was 452.89 μeq/L, with SO42- and NO-3 as the main anions, which accounted for 59.20% and 31.93% of the total anions in precipitation respectively. On the other hand, NH4+ and Ca2+ were the main cations accounting for 39.21% and 33.87% of the total cations in precipitation respectively. The results of neutralizing factor (NF) indicated that NH4+ and Ca2+ were the dominant neutralization substances. The seasonal variations of ions showed that the concentrations were higher in winter than in summer and autumn. The correlation analysis of chemical composition in the precipitation showed that the correlation coefficients between NH4+ , Ca2+ and SO42-, NO-3 were all greater than 0.7, i.e. NH4NO3, Ca(NO3)2, (NH4)2SO4, CaSO4 and NH4HSO4 existed in the atmosphere of Shangluo. The calculation of enrichment factors indicated that SO42- and NO-3 were most of anthropogenic source, Ca2+, Mg2+ and K+ were mainly from the rock weathering of terrigenous source and Cl- was of marine source.
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