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宋佳玲, 浦婷婷, 薛亚楠, 王晨晖, 方学友, 崔立峰.WO3/TiO2光催化剂的制备及光催化产氢性能研究水资源与水工程学报[J].,2017,28(3):55-60
WO3/TiO2光催化剂的制备及光催化产氢性能研究
Preparation and photocatalytic H2-production performance of WO3/TiO2 photocatalyst
  
DOI:10.11705/j.issn.1672-643X.2017.03.11
中文关键词:  TiO2  WO3  半导体复合  光解水制氢
英文关键词:titanium dioxide  tungsten trioxide  semiconductor composite  photocatalysis water splitting
基金项目:国家自然科学基金项目(51528202、51671136)
作者单位
宋佳玲1, 浦婷婷1, 薛亚楠2, 王晨晖3, 方学友1, 崔立峰1 1.上海理工大学 环境与建筑学院 环境与低碳科学研究中心 上海 200093
2.上海理工大学材料科学与工程学院
上海 200093 3.中国石油管道局工程有限公司 河北 廊坊 065000 
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中文摘要:
      针对催化剂TiO2禁带宽度较宽、光响应范围较窄的问题,对TiO2进行改性,采用溶胶凝胶法制备了不同复合比例的WO3/TiO2催化剂以提高TiO2的光催化活性。应用SEM,BET,XRD,UV-Vis,FT-IR等方法对催化剂进行表征,分析了不同复合比对WO3/TiO2样品形貌、晶型、比表面积和产氢速率的影响。当入射波长为300~600 nm,2%WO3/TiO2的吸光度大于TiO2的吸光度,吸收带边红移。通过300 W氙灯照射进行光解水制氢的测试,评价了不同WO3/TiO2样品的光催化分解水产氢活性。结果表明:复合比为2%时,WO3/TiO2的光解水产氢活性最佳,最高可达14 445.3 μmol/(h·g),其产氢速率是TiO2的10倍,同时探讨分析了光催化反应机理。这将在太阳能光解水产氢领域有着广泛的应用前景。
英文摘要:
      In order to enhance the photocatalytic activity of TiO2 which has a wide band gap width but a narrow range in light responsive region, a series of WO3/TiO2 composite photocatalysts with different composite proportions were prepared by a sol-gel method. The prepared samples were characterized by Scanning Electron Microscopy, N2 physical adsorption, X-ray diffraction, UV-visible spectroscopy and Fourier transform infrared spectroscopy. The effects of different composite proportions on the morphology, crystal structure, specific surface area and photocatalytic activity of WO3/TiO2 were investigated. The photocatalytic activity of the samples was evaluated by photo-catalysis water splitting under 300W Xenon lamp. In addition, the reaction mechanism over the composite catalyst was discussed. The results showed that, when λ was 300 to 600 nm, the absorbance of 2%-WO3/TiO2 was greater than the absorbance of TiO2, the absorption band edge was redshifted. As the composite ratio was 2%, the hydrogen photolysis aquatic activity of WO3/TiO2 was the best, with a highest value of 14445.3 μmol/(h·g), concentration of WO3 showed 10 times photocatalytic activity compared to pure TiO2. The photocatalyst technology would have extensive applications in the field of water splitting by solar light.
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