• ▶ 2008-2024年被中国情报信息研究所评价中心评为“中国科技核心期刊”
  • ▶ 2019-2024年连续三届被中国科学院文献情报中心中国科学引文数据库CSCD(核心库)收录
  • ▶ 2021、2023年入编北京大学图书馆《中文核心期刊要目总览》
  • ▶ 2020-2024连续四年入选《科技期刊世界影响力指数(WJCI)报告》
孙亚茹,黄远星.载锰污泥活性炭催化臭氧氧化草酸废水的研究水资源与水工程学报[J].,2016,27(6):101-107
载锰污泥活性炭催化臭氧氧化草酸废水的研究
Research on the catalytic ozonation of oxalic acid in wastewater with manganese loaded sludge activated carbon as catalyst
  
DOI:10.11705/j.issn.1672-643X.2016.06.18
中文关键词:  载锰污泥活性炭  剩余污泥  臭氧  催化氧化  草酸去除  草酸废水处理
英文关键词:manganese-loaded sludge activated  remaining sludge  ozone  catalytic oxidation  oxalic acid removal  oxalicacid wastewater treatment
基金项目:国家自然科学基金项目(51208299); 上海市教育委员会创新基金项目(15ZZ075)
作者单位
孙亚茹,黄远星 (上海理工大学 环境与建筑学院 上海 200093) 
摘要点击次数: 2223
全文下载次数: 1130
中文摘要:
      为研究在催化臭氧化过程中,载锰污泥活性炭对草酸废水降解的催化效果,以及为污泥的资源化探索一条新途径,本实验采用连续流臭氧氧化实验,通过单因素实验方法考察了载锰污泥活性炭催化臭氧化反应的主要影响因素及最佳反应条件,同时对催化臭氧化反应机理进行了探讨。结果表明:在臭氧浓度为5.0 mg/ L,载锰污泥活性炭投加量为100 mg/L, pH值为3.5的最佳反应条件下,60 min内草酸的去除率最高达91.2%。叔丁醇对草酸降解具有抑制作用,催化臭氧化反应符合羟基自由基的反应机制。该方法的处理效果较为明显,对评价催化臭氧法的效果具有较明显的参考价值。
英文摘要:
      In order to study the catalytic effects of manganese-loading sludge activated carbon on oxalic acid wastewater degradation in the catalytic ozonation processes and to explore a new way on resources recovery of sludge, the continuous flow of ozone oxidation methods were conducted in the expereiments, and the main influence factors and the best reaction conditions of manganese loaded sludge activated carbon catalytic ozonation were investigated by the single factor experimental methods, and the reaction mechanisms of catalytic ozonation were discussed. The results demonstrated that the oxalic acid wastewater had the highest removal rate at 91.2% within 60 min under the best reaction conditions of the ozone concentration being 5.0 mg/L, the dosage of manganese loaded sludge activated carbon being 100 mg/L, and the pH being 3.5. Tert-butyl alcohol had inhibitory effects on degradation of oxalic acid, catalytic ozonation conforms to hydroxyl free radical reaction mechanism. The treatment effects of the method was obvious and itis a significant reference to evaluate the effects of catalytic ozonation.
查看全文  查看/发表评论  下载PDF阅读器
关闭