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张晓东, 董 寒, 赵 迪, 崔立峰, 王 欣.金属有机骨架材料Cu3(BTC)2的制备及其光催化性能研究水资源与水工程学报[J].,2015,26(4):35-37
金属有机骨架材料Cu3(BTC)2的制备及其光催化性能研究
Study on preparation and photocatalytic property of metal organic framework material Cu3(BTC)2
  
DOI:10.11705/j.issn.1672-643X.2015.04.007
中文关键词:  金属有机骨架  Cu3(BTC)2  光催化  水处理  罗丹明B
英文关键词:metal organic framework  Cu3(BTC)2  photocatalytic  water treatment  Rhodaming B
基金项目:上海市青年科技英才扬帆计划项目(14YF1409900); 沪江基金研究基地项目(B14003、 D14004)
作者单位
张晓东1, 董 寒1, 赵 迪1, 崔立峰1, 王 欣2 (1.上海理工大学 环境与建筑学院 环境与低碳科学研究中心 上海 200093 2.大连自然博物馆 辽宁 大连 116023) 
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中文摘要:
      以三水硝酸铜为铜源,通过调控水热温度合成出高结晶度的金属有机骨架Cu3(BTC)2材料。采用X射线衍射(XRD)、扫描电子显微镜(SEM)和热重(TG)手段对所制备的样品进行表征,同时以甲基橙和罗丹明B作为目标降解物研究Cu3(BTC)2材料的光催化性能。光催化降解结果显示:Cu3(BTC)2材料对罗丹明B有较好的降解效率,水热温度对Cu3(BTC)2材料的结构及光催化效率影响较大,水热温度为140℃制备的Cu3(BTC)2样品具有较高的光催化效率。这主要是由于高的结晶度可以产生更多的光生电子空穴对和提供更多的反应活性位,这将在处理环境污染物方面有着巨大的潜在的应用前景。
英文摘要:
      Metal organic framework material Cu3(BTC)2 was successfully prepared by using Cu(NO3)2·3H2O as copper source by hydrothermal method.The paper used the means such as XRD, SEM, and TG to characterize the synthesized samples and took methyl orange and Rhodamine B as target degradation substance to study the property of photocatalyst of Cu3(BTC)2. The result indicated that there are better degradation effect of Cu3(BTC)2 material on Loudanming B The hydrothermal temperature has great impact on the structure of Cu3(BTC)2 and photocatalyst effect.The sample Cu3(BTC)2 has higher photocatalytic efficiency when the hydrothermal temperature is 140℃.Which mainly attributes to that the high crystallinity can produce more photogenerated electron hole pairs and reaction active sites. The experiment has broadened development of photocatalyst technology in control field of environment pollution.
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